Capaldi previously performed his global breakthrough hit, 'Someone You Loved' on 'Tonight' in October 2019.
'Once Upon A Time In Hollywood', 'Avengers: Endgame' and 'Chernobyl' were also victorious.
The new collection includes classic tracks from Doris Day, Louis Prima, Nina Simone, and many others.
'The Marvelous Mrs. Maisel' and 'Green Book' also picked up awards at the prestigious annual ceremony.
Greta Van Fleet were recently nominated for three 2019 Grammy Awards, including best new artist and best rock performance for ‘Highway Tune'.
Presented by Andy Samberg and Sandra Oh, the 76th Golden Globes came from the Beverley Hills Hinton in California.